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Size and composition measurements of background aerosol and new particle growth in a Finnish forest during QUEST 2 using an Aerodyne Aerosol Mass Spectrometer

by J. D. Allan, M. R. Alfarra, K. N. Bower, H. Coe, J. T. Jayne, D. R. Worsnop, P. P. Aalto, M. Kulmala, T. Hyötyläinen, F. Cavalli, A. Laaksonen show all authors
Atmospheric Chemistry and Physics Discussions ()

Abstract

The study of the growth of nucleation-mode particles is important, as this prevents their loss through diffusion and allows them to reach sizes where they may become effective cloud condensation nuclei. Hyytiala, a forested site in southern Finland, frequently experiences particle nucleation events during the spring and autumn, where particles first appear during the morning and continue to grow for several hours afterwards. As part of the QUEST 2 intensive field campaign during March and April 2003, an Aerodyne Aerosol Mass Spectrometer (AMS) was deployed alongside other aerosol instrumentation to study the particulate composition and dynamics of growth events and characterise the background aerosol. Despite the small mass concentrations, the AMS was able to distinguish the grown particles in the < 100 nm regime several hours after an event and confirm that the particles were principally organic in composition. The AMS was also able to derive a mass spectral fingerprint for the organic species present, and found that it was consistent between events and independent of the mean particle diameter during non-polluted cases, implying the same species were also condensing onto the accumulation mode. The results were compared with those from offline analyses such as GC-MS and were consistent with the hypothesis that the main components were alkanes from plant waxes and the oxidation products of terpenes.

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