Abstract
MFM-300(Al) shows reversible uptake of NH3 (15.7 mmol g−1 at 273 K and 1.0 bar) over 50 cycles with an exceptional packing density of 0.62 g cm−3 at 293 K. In situ neutron powder diffraction and synchrotron FTIR micro-spectroscopy on ND3@MFM-300(Al) confirms reversible H/D site exchange between the adsorbent and adsorbate, representing a new type of adsorption interaction.
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Godfrey, H. G. W., da Silva, I., Briggs, L., Carter, J. H., Morris, C. G., Savage, M., … Schröder, M. (2018). Ammonia Storage by Reversible Host–Guest Site Exchange in a Robust Metal–Organic Framework. Angewandte Chemie - International Edition, 57(45), 14778–14781. https://doi.org/10.1002/anie.201808316
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