Atmospheric aerosols play a substantial role in climate change through radiative forcing. Combustion-produced carbonaceous particles are the main light-absorbing aerosols; thus, quantifying their optical properties is essential for determining the magnitude of direct forcing. By using the electron energy-loss spectrum in the transmission electron microscope, we quantified the optical properties of individual, submicrometer amorphous carbon spheres that are ubiquitous in East Asian-Pacific outflow. The data indicate that these common spheres are brown, not black, with a mean refractive index of 1.67 - 0.27i (where i = √1) at a wavelength of 550 nanometers. The results suggest that brown carbon aerosols should be explicitly included in radiative forcing models.
CITATION STYLE
Alexander, D. T. L., Crozier, P. A., & Anderson, J. R. (2008). Brown carbon spheres in East Asian outflow and their optical properties. Science, 321(5890), 833–836. https://doi.org/10.1126/science.1155296
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