Metal-free Bronsted acid catalyzed transfer hydrogenation: enantioselective synthesis of tetrahydroquinolines.

  • Rueping M
  • Theissmann T
  • Antonchick A
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Abstract

Diphenylphosphate catalyzes the metal-free redn. of ketimines under hydrogen-transfer conditions with Hantzsch dihydropyridine as the hydrogen source. The asym. variant of this procedure using 1 mol % of a chiral BINOL-phosphate I as catalyst is reported. [on SciFinder(R)]

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Rueping, M., Theissmann, T., & Antonchick, A. P. (2007). Metal-free Bronsted acid catalyzed transfer hydrogenation: enantioselective synthesis of tetrahydroquinolines. In Catal. Fine Chem. Synth. (Vol. 5, pp. 170–176). John Wiley & Sons Ltd.

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