Charge and heat transport through quantum dots with local and correlated-hopping interactions

Abstract

The transport properties of junctions composed of a central region tunnel-coupled to external electrodes are frequently studied within the single-impurity Anderson model with Hubbard on-site interaction. In the present work, we supplement the model with an important ingredient, namely, the charge-bond interaction, also known as correlated or assisted hopping. Correlated hopping enters the second-quantized Hamiltonian, written in the Wannier representation, as an off-diagonal many-body term. Using the equation of motion technique, we study the effect of the correlated hopping on the spectral and transport characteristics of a two-terminal quantum dot. Two different Green functions (GFs) appear: one of them describes the spectral properties of the quantum dot, the other the transport properties of the system. The calculation of the transport GF requires the knowledge of the spectral one. We use decoupling procedures similar to those which properly describe the standard Anderson model within the Kondo regime and outside of it. For an arbitrary ratio between the amplitudes of correlated and single-particle hopping terms, the transport GF fulfils the symmetry of the model. The average occupation of the dot also obeys this symmetry, albeit the spectral function of the quantum dot, calculated within an analogous decoupling scheme as for the transport GF, does not. We identify the physical reason for this behavior and propose a way to cure it. Since the correlated-hopping term breaks the particle-hole symmetry of the model and modifies all transport characteristics of the system, the detailed knowledge of its influence on measurable characteristics is a prerequisite for its experimental detection. Simple, experimentally feasible methods are proposed.