Ultrathin Bi2O2Se/Si Heterojunction Photodetector with Tunneling Oxide Passivation for Enhanced Optoelectronic Performance

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Abstract

Two-dimensional (2D) materials have garnered significant attention for next-generation optoelectronic devices due to their exceptional physical properties. This study introduces a high-performance ultrathin Bi2O2Se/Si heterojunction photodetector with tunneling oxide passivation, fabricated using a transfer-free pulsed laser deposition method. The Bi2O2Se layer exhibits strong air stability and compatibility for practical applications. By incorporating a thin SiO2 tunneling layer, the heterostructure achieves a low dark current (∼22.3 nA/cm2), a high on/off ratio (∼8 × 106), and a responsivity of 23.0 A/W. Compared to traditional CdS/Si devices, this photodetector demonstrates superior performance, including faster response time and higher stability. These findings underscore the potential of Bi2O2Se/Si heterostructures for advanced photonic and optoelectronic applications.

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APA

Hung, T. P., Chen, W. H., Chen, Y. J., Tu, Y. H., Huang, Z. H., Chueh, Y. L., … Chen, C. Y. (2025). Ultrathin Bi2O2Se/Si Heterojunction Photodetector with Tunneling Oxide Passivation for Enhanced Optoelectronic Performance. ACS Applied Materials and Interfaces, 17(18), 26931–26939. https://doi.org/10.1021/acsami.5c03477

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