Measurement report: Impact of African aerosol particles on cloud evolution in a tropical montane cloud forest in the Caribbean

Abstract

African aerosol particles, traveling thousands of kilometers before reaching the Americas and the Caribbean, directly scatter and absorb solar radiation and indirectly impact climate by serving as cloud condensation nuclei (CCN) or ice-nucleating particles (INPs) that form clouds. These particles can also affect the water budget by altering precipitation patterns that subsequently affect ecosystems. As part of the NSF-funded Luquillo Critical Zone Observatory, field campaigns were conducted during the summers of 2013 (23 d), 2014 (11 d), and 2015 (92 d) at Pico del Este, a site in a tropical montane cloud forest on the Caribbean Island of Puerto Rico. Cloud microphysical properties, which included liquid water content, droplet number concentration, and droplet size, were measured. Using products from models and satellites, as well as in situ measurements of aerosol optical properties, periods of high-and low-dust influence were identified. The results from this study suggest that meteorology and air mass history have a more important effect on cloud processes than aerosols transported from Africa. In contrast, air masses that arrived after passing over the inhabited islands to the southeast led to clouds with much higher droplet concentrations, presumably due to aerosols formed from anthropogenic emissions.