Increasing the impact toughness of cellulose fiber reinforced polypropylene composites—influence of different impact modifiers and production scales

Abstract

While cellulose fiber reinforced polypropylene (PP) composites typically offer good stiffness and strength in combination with ecological benefits and a high potential for lightweight construction, they often require measures taken to improve their impact performance. In this work, the influence of different types of impact modifier on the mechanical performance of a PP–cellulose composite was systematically investigated, with a particular focus on the improvement of the notched impact strength and the accompanying loss of stiffness. Among the tested impact modifiers, ethylene-octene copolymers appeared to be the most suitable class to achieve a good overall performance. A high modifier viscosity increased its potential to improve the notched impact strength of the composite. Additionally, composite production on a larger scale improved the impact performance without significantly affecting the tensile properties. Several composites from this study surpassed the overall mechanical performance of a benchmark commercial PP–cellulose composite. While the impact strength of commercial high-impact PP–talc composites could not be reached, the considerably lower density of the PP–cellulose composites is worth mentioning.