Multiscale micromechanics modeling of plant fibers: upscaling of stiffness and elastic limits from cellulose nanofibrils to technical fibers

Abstract

The mechanical properties of natural fibers, as used to produce sustainable biocomposites, vary significantly—both among different plant species and also within a single species. All plants, however, share a common microstructural fingerprint. They are built up by only a handful of constituents, most importantly cellulose. Through continuum micromechanics multiscale modeling, the mechanical behavior of cellulose nanofibrils is herein upscaled to the technical fiber level, considering 26 different commonly used plants. Model-predicted stiffness and elastic limit bounds, respectively, frame published experimental ones. This validates the model and corroborates that plant-specific physicochemical properties, such as microfibril angle and cellulose content, govern the mechanical fiber performance.