Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe 2 mediated by mode-selective electron-phonon coupling

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Abstract

Quantum materials represent one of the most promising frontiers in the quest for faster, lightweight, energy-efficient technologies. However, their inherent complexity and rich phase landscape make them challenging to understand or manipulate. Here, we present a new ultrafast electron calorimetry technique that can systematically uncover new phases of quantum matter. Using time- and angle-resolved photoemission spectroscopy, we measure the dynamic electron temperature, band structure, and heat capacity. This approach allows us to uncover a new long-lived metastable state in the charge density wave material 1T-TaSe 2 , which is distinct from all the known equilibrium phases: It is characterized by a substantially reduced effective total heat capacity that is only 30% of the normal value, because of selective electron-phonon coupling to a subset of phonon modes. As a result, less energy is required to melt the charge order and transform the state of the material than under thermal equilibrium conditions.

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Shi, X., You, W., Zhang, Y., Tao, Z., Oppeneer, P. M., Wu, X., … Murnane, M. (2019). Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe 2 mediated by mode-selective electron-phonon coupling. Science Advances, 5(3). https://doi.org/10.1126/sciadv.aav4449

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