Polaron relaxation in a quantum dot due to anharmonic coupling within a mean-field approach

Abstract

We study the electronic relaxation in a quantum dot within the polaron approach by focusing on the reversible anharmonic decay of longitudinal optical (LO) phonons forming the polaron into longitudinal-acoustic (LA) phonons. The coherent coupling between the LO and LA phonons is treated within a mean-field approach. We derive a temperature-dependent interlevel coupling parameter, related to the Grüneisen parameter and the thermal-expansion coefficient, which characterizes an effective decay channel for the electronic (or excitonic) states. Within this theory, we obtain a characteristic anharmonic decay time of 1 ns, 2-3 orders of magnitude longer than previous predictions based on the Fermi's Golden Rule. We suggest that coherent relaxation due to carrier-carrier interaction is an efficient alternative to the (too slow) polaron decay. © 2009 The American Physical Society.