Thermal, photonic, and electrocatalysis in lignin depolymerization research

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Abstract

In order to realize a sustainable bio-based future, it is essential to fully harness the potential of biomass, including lignin - a readily available biopolymer that ranks second in abundance and serves as a renewable source of aromatics. While lignin has traditionally been used for lower-value applications like fuel and power generation, unlocking its higher-value potential through diverse conversion and upgrading techniques is of paramount importance. This review focuses on the catalytic conversion of lignin, with a specific emphasis on selective depolymerization, a process that not only supports economically and environmentally sustainable biorefineries but also aligns with Green Chemistry principles, mitigating adverse environmental impacts. Furthermore, we provide a comprehensive discussion of reaction pathways and mechanisms, including C-O and C-C bond cleavage, among different catalysts. Lastly, we analyze and briefly discuss the prospects of rational catalyst design in biomass valorization.

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Ziwei, W., Hao, S., Yizhen, C., Ben, L., Yaowei, X., Wanxia, W., … Lei, W. (2023, November 6). Thermal, photonic, and electrocatalysis in lignin depolymerization research. RSC Advances. Royal Society of Chemistry. https://doi.org/10.1039/d3ra06880c

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