Assessment of the applicability of a low-cost sensor–based methane monitoring system for continuous multi-channel sampling

Abstract

Systems that are made of several low-cost gas sensors with automatic gas sampling may have the potential to serve as reliable fast methane analyzers. However, there is a lack of reports about such types of systems evaluated under field conditions. Here, we developed a continuous methane monitoring system with automated gas sampling unit using low-cost gas sensors, TGS 2611 and MQ-4, that use a simple cloud-based data acquisition platform. We verified the consistency, repeatability, and reproducibility of the data obtained by TGS 2611 and MQ-4 low-cost gas sensors by measuring high- and low-concentration methane samples. The normalized root-mean-square errors (NRMSEs) of the samples with high methane concentrations, [CH4] of 3, 4, 6, and 7%, were 0.0788, 0.0696, 0.1198, and 0.0719 for the TGS 2611 sensor, respectively, and were confirmed using a gas chromatograph as a reference analyzer. The NRMSEs of the samples with low [CH4] of 0.096, 0.145, 0.193, and 0.241% measured by the TGS 2611 sensor were 0.0641, 0.1749, 0.0157, and 0.1613, whereas those NRMSEs of the same concentrations measured by the MQ-4 sensor were 0.3143, 0.5766, 0.6301, and 0.6859, respectively. Laboratory-scale anaerobic digesters were tested using the developed system. The anaerobic digesters were continuously operated for 2 months, demonstrating the potential use of sensors for detecting and monitoring methane in the field level application. This study utilized a unique way to combine the advantages of low-cost sensors and develop a reliable monitoring system by minimizing drawbacks of low-cost sensors.