Effect of Interface Modification on Mechanoluminescence-Inorganic Perovskite Impact Sensors

Abstract

It is becoming increasingly important to develop innovative self-powered, low-cost, and flexible sensors with the potential for structural health monitoring (SHM) applications. The mechanoluminescence (ML)-perovskite sensor is a potential candidate that combines the light-emitting principles of mechanoluminescence with the light-absorbing properties of perovskite materials. Continuous in-situ SHM with embedded sensors necessitates long-term stability. A highly stable cesium lead bromide photodetector with a carbon-based electrode and a zinc sulfide (ZnS): copper (Cu) ML layer was described in this article. The addition of a magnesium iodide (MgI2) interfacial modifier layer between the electron transport layer (ETL) and the Perovskite interface improved the sensor’s performance. Devices with the modified structure outperformed devices without the addition of MgI2 in terms of response time and impact-sensing applications.