Nonadiabatic multielectron dynamics in strong field molecular ionization

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Abstract

The limits of the quasistatic tunnel ionization model in unsaturated linear hydrocarbons were systematically studied. A new ionization dynamics was observed that is due to nonadiabatic multielectron (NME) excitations during the ionization process. The resulting excitation and ionization lead to very strong fragmentation with important consequences for many applications of intense femtosecond pulses.

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Lezius, M., Blanchet, V., Rayner, D. M., Villeneuve, D. M., Stolow, A., & Ivanov, M. Y. (2001). Nonadiabatic multielectron dynamics in strong field molecular ionization. Physical Review Letters, 86(1), 51–54. https://doi.org/10.1103/PhysRevLett.86.51

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