Significant impact of the East Asia monsoon on ozone seasonal behavior in the boundary layer of Eastern China and the west Pacific region

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Abstract

The impact of the East Asia monsoon on the seasonal behavior of O 3 in the boundary layer of Eastern China and the west Pacific region was analyzed for 2004-2006 by means of full-year nested chemical transport model simulations and continuous observational data obtained from three inland mountain sites in central and eastern China and three oceanic sites in the west Pacific region. The basic common features of O 3 seasonal behaviors over all the monitoring sites are the pre-and post-monsoon peaks with a summer trough. Such bimodal seasonal patterns of O 3 are predominant over the region with strong summer monsoon penetration, and become weaker or even disappear outside the monsoon region. The seasonal/geographical distribution of the pre-defined monsoon index indicated that the East Asia summer monsoon is responsible for the bimodal seasonal O 3 pattern, and also partly account for the differences in the O 3 seasonal variations between the inland mountain and oceanic sites. Over the inland mountain sites, the O 3 concentration increased gradually from the beginning of the year, reached a maximum in June, decreased rapidly to the summer valley in July or August, and then peaked in September or October, thereafter decreased gradually again. Over the oceanic sites, O 3 abundance showed a similar increasing trend beginning in January, but then decreased gradually from the end of March, followed by a wide trough with the minimum in July and August and a small peak in October or November. A sensitivity analysis performed by setting China-emission to zero revealed that the chemically produced O 3 from China-emission contributed substantially to the O 3 abundance, particularly the pre-and post-monsoon O 3 peaks, over China mainland. We found that China-emission contributed more than 40% to total boundary layer O 3 during summertime (60-70% in July) and accounted for about 40ppb of each peak value over the inland region if without considering the effect of the nonlinear chemical productions. In contrast, over the oceanic region in the high monsoon index zone, the contribution of China-emission to total boundary layer O 3 was always less than 20% ( < 10 ppb), and less than 10% in summer. © Author(s) 2008.

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APA

He, Y. J., Uno, I., Wang, Z. F., Pochanart, P., Li, J., & Akimoto, H. (2008). Significant impact of the East Asia monsoon on ozone seasonal behavior in the boundary layer of Eastern China and the west Pacific region. Atmospheric Chemistry and Physics, 8(24), 7543–7555. https://doi.org/10.5194/acp-8-7543-2008

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