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Abstract

We have combined a Stark decelerator with a molecular beam-surface scattering setup to accurately measure the absolute electron emission yield, γ, of CO (a(3)Π) quenching at a Au(111) surface with quantum state resolution. We clearly observe an enhanced probability of electron emission when scattering vibrationally excited states of CO from the surface.

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Grätz, F., Engelhart, D. P., Wagner, R. J. V., Haak, H., Meijer, G., Wodtke, A. M., & Schäfer, T. (2013). Vibrational enhancement of electron emission in CO (a3Π) quenching at a clean metal surface. Physical Chemistry Chemical Physics, 15(36), 14951–14955. https://doi.org/10.1039/c3cp52468j

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