Modelling forced periodic operation of catalytic reactors

  • Feimer J
  • Jain A
  • Hudgins R
 et al. 
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Abstract

The kinetic adsorption/desorption or AD models used to predict product selectivities obtained through forced-feed concentration cycling have been re-examined. Selectivity improvement results from model structure and nonlinear rates of reaction. The relaxed-steady state bound to periodic operation was found to be predictable from steady state rates for the kinetic model used. Adsorption/desorption models predict no rate improvement for periodic operation. Also they fail to predict experimental observations that are now fairly extensive. © 1982.

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Authors

  • J. L. Feimer

  • A. K. Jain

  • R. R. Hudgins

  • P. L. Silveston

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