Optical excitations in a quarter-filled Ni(dmit)2based compound described by a dimerized octamer model

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Abstract

The reflectance spectra of [SMe3][Ni(dmit)2(dmit = 1,3-dithiole-2 thione-4,5-dithiolato), quarter-filled organic conductor with strongly dimerized structure, will be discussed in the framework of the new Raman results for this compound. The spectra are interpreted on the basis of a dimerized Hubbard octamer model, which accounts for the low energy electronic transitions and for the coupling of the electronic excitations with the intramolecular vibrations.

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Pokhodnya, K. I., Cassoux, P., Feltre, L., & Meneghetti, M. (1999). Optical excitations in a quarter-filled Ni(dmit)2based compound described by a dimerized octamer model. Synthetic Metals, 103(1–3), 2187. https://doi.org/10.1016/S0379-6779(98)00860-1

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