Magnetic nanomaterials are considered, formed by magnetic nanomolecules with high spins. The problem of spin reversal in these materials is analyzed, which is of interest for the possible use of such materials for quantum information processing and quantum computing. The fastest spin reversal can be achieved by coupling the spin sample to a resonant electric circuit and by an appropriate choice of the system parameters. A principal point is to choose these parameters so that to organize coherent spin motion. Dynamics of collective motion is modelled by computer simulations, which confirm the high level of dynamical coherence of molecular spins in the process of spin reversal.
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