Atmospheric Chemistry and Physics, vol. 13, issue 8 (2013) pp. 3899-39808 Published by Copernicus GmbH
Improved characterization of aerosol properties in the vicinity of clouds is important for better understanding two critical aspects of climate: aerosol-cloud interactions and the direct radiative effect of aerosols. Satellite measurements have provided important insights into aerosol properties near clouds, but also suggested that the observations can be affected by 3-D radiative processes and instrument blurring not considered in current data interpretation methods. This study examines systematic cloud-related changes in particle properties and radiation fields that influence satellite measurements of aerosols in the vicinity of low-level maritime clouds. For this, the paper presents a statistical analysis of a yearlong global dataset of co-located MODIS and CALIOP observations and theoretical simulations. The results reveal that CALIOP-observed aerosol particle size and optical thickness, and MODIS-observed solar reflectance increase systematically in a wide transition zone around clouds. It is estimated that near-cloud changes in particle populations - including both aerosols and undetected cloud particles - are responsible for roughly two thirds of the observed increase in 0.55 μm MODIS reflectance. The results also indicate that 3-D radiative processes significantly contribute to near-cloud reflectance enhancements, while instrument blurring contributes significantly only within 1 km from clouds and then quickly diminishes with distance from clouds. © Author(s) 2013.
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