Photocatalytic hydrogen production from water using porous material [Ru2(p-BDC)2]n

  • Kataoka Y
  • Sato K
  • Miyazaki Y
 et al. 
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Abstract

We have detected the first example of open porous metal-org. frameworks (MOFs) that functions as an activity site for the redn. of water into hydrogen mols. in the presence of Ru(bpy)32+, MV2+, and EDTA-2Na under visible light irradn. This activity is highly efficient: the turnover no. based on MOFs and the apparent quantum yield are 8.16 and 4.82%, resp. Furthermore, this material enables the adsorption of various gases into its pores; its hydrogen uptake capacity is 1.2 wt% at 77.4 K. [on SciFinder(R)]

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Authors

  • Yusuke Kataoka

  • Konomi Sato

  • Yuhei Miyazaki

  • Kazuki Masuda

  • Hiroshi Tanaka

  • Shuichi Naito

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