Journal article

The response of surface ozone to climate change over the Eastern United States

Racherla P, Adams P ...see all

Atmos. Chem. Phys., vol. 8, issue 4 (2008) pp. 871-885 Published by Copernicus Publications

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We investigate the response of surface ozone (O3) to future climate change in the eastern United States by performing simulations corresponding to present (1990s) and future (2050s) climates using an integrated model of global climate, tropospheric gas-phase chemistry, and aerosols. A future climate has been imposed using ocean boundary conditions corresponding to the IPCC SRES A2 scenario for the 2050s decade. Present-day anthropogenic emissions and CO2/CH4 mixing ratios have been used in both simulations while climate-sensitive emissions were allowed to vary with the simulated climate. The severity and frequency of O3 episodes in the eastern U.S. increased due to future climate change, primarily as a result of increased O3 chemical production. The 95th percentile O3 mixing ratio increased by 5 ppbv and the largest frequency increase occured in the 80–90 ppbv range; the US EPA's current 8-h ozone primary standard is 80 ppbv. The increased O3 chemical production is due to increases in: 1) natural isoprene emissions; 2) hydroperoxy radical concentrations resulting from increased water vapor concentrations; and, 3) NOx concentrations resulting from reduced PAN. The most substantial and statistically significant (p

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  • P N Racherla

  • P J Adams

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