Rh(iii)-Catalyzed intramolecular redox-neutral cyclization of alkenes via C-H activation

  • Shi Z
  • Boultadakis-Arapinis M
  • Koester D
 et al. 
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Abstract

Biologically interesting fused oligocyclic lactams have been prepared via an intramolecular redox-neutral cyclization process. By the proper choice of the substrates with a wide variety of tethered olefins, the less favored C-H bond can be activated and functionalized. This C-H activation proceeds under mild conditions, obviates the need for external oxidants, and displays a broad scope with respect to the substituents. ? The Royal Society of Chemistry 2014.

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Authors

  • Zhuangzhi Shi

  • Mélissa Boultadakis-Arapinis

  • Dennis C. Koester

  • Frank Glorius

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