Atmospheric Chemistry and Physics, vol. 13, issue 6 (2013) pp. 3307-3319 Published by European Geosciences Union
Measurements of mixing ratio profiles of stratospheric bromine monoxide (BrO) were made using observations of BrO rotational line emission at 650.179 GHz by a balloon-borne SIS (superconductor-insulator-superconductor) submillimeterwave heterodyne limb sounder (SLS). The balloon was launched from Ft. Sumner, New Mexico (34 degrees N) on 22 September 2011. Peak mid-day BrO abundance varied from 16 +/- 2 ppt at 34 km to 6 +/- 4 ppt at 16 km. Corresponding estimates of total inorganic bromine (Br-y), derived from BrO vmr (volume mixing ratio) using a photochemical box model, were 21 +/- 3 ppt and 11 +/- 5 ppt, respectively. Inferred Br-y abundance exceeds that attributable solely to decomposition of long-lived methyl bromide and other halons, and is consistent with a contribution from bromine-containing very short lived substances, Br-y(VSLS), of 4 ppt to 8 ppt. These results for BrO and Br-y were compared with, and found to be in good agreement with, those of other recent balloon-borne and satellite instruments.
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