The AgGaSe2as well as AgGaS2has been showed to be efficient frequency doubling crystals for infrared radiation such as the 10.6 μm CO2laser. The production of these crystals needs good knowledge of the phase relationship. The thermodynamic description of the binary Ag-Ga system has been chosen as a first step for the description of the Ag-Ga-Se and Ag-Ga-S systems. The Calphad approach has been used for this modeling. Good agreement between experimental data and calculated values has been found. © 2010 Elsevier B.V. All rights reserved.
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