Journal article

A tropospheric ozone maximum over the equatorial Southern Indian Ocean

Zhang L, Li Q, Murray L, Luo M, Liu H, Jiang J, Mao Y, Chen D, Gao M, Livesey N ...see all

Atmospheric Chemistry and Physics, vol. 12, issue 9 (2012) pp. 4279-4296

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We examine the distribution of tropical tropospheric ozone (O-3) from
the Microwave Limb Sounder (MLS) and the Tropospheric Emission
Spectrometer (TES) by using a global three-dimensional model of
tropospheric chemistry (GEOS-Chem). MLS and TES observations of
tropospheric O-3 during 2005 to 2009 reveal a distinct, persistent O-3
maximum, both in mixing ratio and tropospheric column, in May over the
Equatorial Southern Indian Ocean (ESIO). The maximum is most pronounced
in 2006 and 2008 and less evident in the other three years. This feature
is also consistent with the total column O-3 observations from the Ozone
Mapping Instrument (OMI) and the Atmospheric Infrared Sounder (AIRS).
Model results reproduce the observed May O-3 maximum and the associated
interannual variability. The origin of the maximum reflects a complex
interplay of chemical and dynamic factors. The O-3 maximum is dominated
by the O-3 production driven by lightning nitrogen oxides (NOx)
emissions, which accounts for 62% of the tropospheric column O-3 in May
2006. We find the contribution from biomass burning, soil, anthropogenic
and biogenic sources to the O-3 maximum are rather small. The O-3
productions in the lightning outflow from Central Africa and South
America both peak in May and are directly responsible for the O-3
maximum over the western ESIO. The lightning outflow from Equatorial
Asia dominates over the eastern ESIO. The interannual variability of the
O-3 maximum is driven largely by the anomalous anti-cyclones over the
southern Indian Ocean in May 2006 and 2008. The lightning outflow from
Central Africa and South America is effectively entrained by the
anti-cyclones followed by northward transport to the ESIO.

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  • L. Zhang

  • Q. B. Li

  • L. T. Murray

  • M. Luo

  • H. Liu

  • J. H. Jiang

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