Two-dimensional metal-organic frameworks for energy-related electrocatalytic applications

Abstract

In this short perspective we examine recent developments in the design, synthesis and use of metal-organic frameworks (MOFs) for electrocatalytic applications. We discuss the inherent challenges and limitations that continue to plague conventional MOFs and novel strategies for overcoming them. In particular we focus on the growing interest in two-dimensional MOFs as a practical HER/OER/NRR/CO2RR catalyst. We also consider its exciting value as a tool for probing the underlying reaction mechanism and catalytic function of various metals.