Nuclear data uncertainty quantification in criticality safety evaluations for spent nuclear fuel geological disposal

Abstract

Presently, a criticality safety evaluation methodology for the final geological disposal of Swiss spent nuclear fuel is under development at the Paul Scherrer Institute in collaboration with the Swiss National Technical Competence Centre in the field of deep geological disposal of radioactive waste. This method in essence pursues a best estimate plus uncertainty approach and includes burnup credit. Burnup credit is applied by means of a computational scheme called BUCSS-R (Burnup Credit System for the Swiss Reactors–Repository case) which is complemented by the quantification of uncertainties from various sources. BUCSS-R consists in depletion, decay and criticality calculations with CASMO5, SERPENT2 and MCNP6, respectively, determining the keff eigenvalues of the disposal canister loaded with the Swiss spent nuclear fuel assemblies. However, the depletion calculation in the first and the criticality calculation in the third step, in particular, are subject to uncertainties in the nuclear data input. In previous studies, the effects of these nuclear data-related uncertainties on obtained keff values, stemming from each of the two steps, have been quantified independently. Both contributions to the overall uncertainty in the calculated keff values have, therefore, been considered as fully correlated leading to an overly conservative estimation of total uncertainties. This study presents a consistent approach eliminating the need to assume and take into account unrealistically strong correlations in the keff results. The nuclear data uncertainty quantification for both depletion and criticality calculation is now performed at once using one and the same set of perturbation factors for uncertainty propagation through the corresponding calculation steps of the evaluation method. The present results reveal the overestimation of nuclear data-related uncertainties by the previous approach, in particular for spent nuclear fuel with a high burn-up, and underline the importance of consistent nuclear data uncertainty quantification methods. However, only canister loadings with UO2 fuel assemblies are considered, not offering insights into potentially different trends in nuclear data-related uncertainties for mixed oxide fuel assemblies.