We observe time-domain coherent vibrational wavepackets at 1585-cm-1 frequency (21-fs period) using broadband probe pulses strongly chirped up to 150-fs duration. The results are explained using the chronocyclic (Wigner) representation of the chirped pulse.
CITATION STYLE
Polli, D., Brida, D., Lanzani, G., & Cerullo, G. (2009). Observation of High-Frequency Coherent Vibrational Motion with Strongly Chirped Probe Pulses. In Springer Series in Chemical Physics (Vol. 92, pp. 337–339). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_109
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