Abstract
We observe tight and loose ion pairs in bimolecular electron transfer with ultrafast infrared spectroscopy. For large exergonicity tight donor-acceptor pairs do not rearrange into loose complexes before the reaction proceeds, contrasting generally accepted models.
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Mohammed, O. F., Adamczyk, K., Banerji, N., Dreyer, J., Lang, B., Nibbering, E. T. J., & Vauthey, E. (2009). Direct Femtosecond Observation of Tight and Loose Ion Pairs upon Photoinduced Bimolecular Electron Transfer. In Springer Series in Chemical Physics (Vol. 92, pp. 613–615). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_199
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