Ultrabroadband photosensitivity from visible to terahertz at room temperature

Abstract

Charge density wave (CDW) is one of the most fundamental quantum phenomena in solids. Different from ordinary metals in which only single-particle excitations exist, CDW also has collective excitations and can carry electric current in a collective fashion. Manipulating this collective condensation for applications has long been a goal in the condensed matter and materials community. We show that the CDW system of 1T-TaS2 is highly sensitive to light directly from visible down to terahertz, with current responsivities on the order of ~1 AW−1 at room temperature. Our findings open a new avenue for realizing uncooled, ultrabroadband, and sensitive photoelectronics continuously down to the terahertz spectral range.