The change in the low frequency (0.1 - 500 cm-1) non-resonant Raman response following excitation of a dye molecule in solution has been measured as a function of time after resonant excitation of a solute using a two-dimensional mixed resonant, non-resonant time domain spectroscopy. This method provides a direct measurement of the change in the spectrum of the local environment as a dynamic event proceeds in a condensed phase.
CITATION STYLE
Underwood, D. F., & Blank, D. A. (2004). Time resolved direct probing of the change in the local solvent response following excitation of a solute. In Springer Series in Chemical Physics (Vol. 79, pp. 413–415). https://doi.org/10.1007/3-540-27213-5_127
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