A remote sensing technique for global monitoring of power plant CO 2 emissions from space and related applications

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Abstract

Carbon dioxide (CO 2) is the most important anthropogenic greenhouse gas (GHG) causing global warming. The atmospheric CO 2 concentration increased by more than 30% since pre-industrial times - primarily due to burning of fossil fuels - and still continues to increase. Reporting of CO 2 emissions is required by the Kyoto protocol. Independent verification of reported emissions, which are typially not directly measured, by methods such as inverse modeling of measured atmospheric CO 2 concentrations is currently not possible globally due to lack of appropriate observations. Existing satellite instruments such as SCIAMACHY/ENVISAT and TANSO/GOSAT focus on advancing our understanding of natural CO 2 sources and sinks. The obvious next step for future generation satellites is to also constrain anthropogenic CO 2 emissions. Here we present a promising satellite remote sensing concept based on spectroscopic measurements of reflected solar radiation and show, using power plants as an example, that strong localized CO 2 point sources can be detected and their emissions quantified. This requires mapping the atmospheric CO 2 column distribution at a spatial resolution of 2×2 km 2 with a precision of 0.5% (2 ppm) or better. We indicate that this can be achieved with existing technology. For a single satellite in sun-synchronous orbit with a swath width of 500 km, each power plant (PP) is overflown every 6 days or more frequent. Based on the MODIS cloud mask data product we conservatively estimate that typically 20 sufficiently cloud free overpasses per PP can be achieved every year. We found that for typical wind speeds in the range of 2-6 m/s the statistical uncertainty of the retrieved PP CO 2 emission due to instrument noise is in the range 1.6-4.8 MtCO 2/yr for single overpasses. This corresponds to 12-36% of the emission of a mid-size PP (13 MtCO 2/yr). We have also determined the sensitivity to parameters which may result in systematic errors such as atmospheric transport and aerosol related parameters. We found that the emission error depends linearly on wind speed, i.e., a 10% wind speed error results in a 10% emission error, and that neglecting enhanced aerosol concentrations in the PP plume may result in errors in the range 0.2-2.5 MtCO 2/yr, depending on PP aerosol emission. The discussed concept has the potential to contribute to an independent verification of reported anthropogenic CO 2 emissions and therefore could be an important component of a future global anthropogenic GHG emission monitoring system. This is of relevance in the context of Kyoto protocol follow-on agreements but also allows detection and monitoring of a variety of other strong natural and anthropogenic CO 2 and CH 4 emitters. The investigated instrument is not limited to these applications as it has been specified to also deliver the data needed for global regional-scale CO 2 and CH 4 surface flux inverse modeling. © 2010 Author(s).

Figures

  • Fig. 1. Left: Simulation of the atmospheric CO2 column enhancement due to CO2 emission of a power plant using a quasi-stationary Gaussian plume model. The power plant location is indicated by the black cross. A value of 1.0 (green) corresponds to the background CO2 column. A value of 1.02 (red) corresponds to a column enhancement of 2% or larger relative to the background. The wind speed is 1 m/s. The assumed power plant emission is 13 MtCO2/yr corresponding to a power plant such as Schwarze Pumpe located in eastern Germany near Berlin (see photo taken during an overflight with the MAMAP aircraft instrument). Right: as left hand side but at a spatial resolution of 2×2 km2 obtained by box-car averaging the high resolution plume shown on the left hand side. The inlet shows MAMAP CO2 column retrievals around the location of the power plant Schwarze Pumpe (see main text and Fig. 2 for details). The maximum value of the CO2 normalized column is 1.126 for the high resolution plume on the left (resolution 20×20 m2) and 1.031 for the 2×2 km2 resolution plume shown on the right. To better visualize the extent of the CO2 plumes values below 1.0025 are shown in white (see also the black vertical line in the color bar).
  • Table 1. Maximum CO2 column enhancement (relative to background column (=1.0)) for a power plant emitting 13 MtCO2/yr for different spatial resolutions of the satellite footprint. The assumed wind speed is 1 m/s.
  • Fig. 2. (a) Normalized CO2 columns as retrieved from MAMAP aircraft observations on 26 July 2007. The CO2 columns have been normalized by simultaneously retrieved CH4 columns. (b) Retrieved CO2 columns without normalization by CH4. (c) Retrieved CH4 columns. The black cross indicates the location of the power plant Schwarze Pumpe (latitude 51.54◦ N, longitude 14.35◦ E), Germany. The blue arrows indicate the approximate wind direction, which changed during the time of the measurements.
  • Fig. 3. Signal-to-noise ratios (SNRs) as a function of the radiance as measured by CarbonSat in nadir mode for the eight scenarios listed in Table 3 The black crosses show the SNRs computed using the instrument model described in Sect. 5.1. The red squares show the SNRs which can be obtained in the shot noise limit (SNR= √ S).
  • Fig. 4. Results of the CarbonSat instrument simulation for the VEG 50 scenario (albedo: vegetation, SZA 50◦) for an integration time of tint = 0.3 s. Top: Radiance spectra in the three spectral bands covered by CarbonSat. Middle: corresponding signal (in electrons; red: before calibration; black: after calibration, i.e., after subtraction of detector dark and thermal background radiation signals). Bottom: corresponding signal-to-noise ratio.
  • Table 2. CarbonSat’s spectral bands, assumed performance parameters and corresponding signal-to-noise ratios (SNRs). Each band is assumed to be equipped with a Focal Plane Array (FPA) with 1000×250 detector pixels in the spectral and spatial directions, respectively. The spectral resolution is specified in terms of the Full Width at Half Maximum (FWHM) of the spectrometer’s line shape function. The spectral sampling ratio, Nsr, is the number of detector pixels per FWHM. The SNR refers to the continuum SNR outside strong absorption lines for nadir measurements with an integration time of tint=0.3 s and for a ground pixel size of 4 km 2. The assumed orbit altitude is 800 km. The SNRs are given for 8 scenarios which differ by surface albedo and solar zenith angle (SZA) (see also Table 3).
  • Fig. 5. A-priori (black) and perturbed (green) CO2 mixing ratio vertical profiles used for the simulated CarbonSat measurements. The solid green line corresponds to the CO2 mixing ratio profile at a distance of 1.41 km from the power plant (as shown by the annotation the XCO2 is enhanced by 1.08% relative to the background XCO2, which is 390.0 ppm), the dotted green profile corresponds to a distance of 2.24 km from the power plant. The assumed power plant emission is F=13 MtCO2/yr and the assumed wind speed is u= 2m/s.
  • Table 3. Specification of eight scenarios and corresponding retrieval precisions for CO2 and CH4 columns, surface pressure (po), XCO2(po) andXCO2(CH4) for CarbonSat nadir mode observations. XCO2(po) refers toXCO2 obtained using the “po-proxy method” andXCO2(CH4) refers toXCO2 obtained using the “CH4-proxy method” (see main text for details). Aerosol scenario: single scattering albedo 0.999, HenyeyGreenstein phase function with asymmetry parameter 0.7, aerosol optical depth (AOD) 0.2 at 550 nm with λ−1 wavelength dependence.

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APA

Bovensmann, H., Buchwitz, M., Burrows, J. P., Reuter, M., Krings, T., Gerilowski, K., … Erzinger, J. (2010). A remote sensing technique for global monitoring of power plant CO 2 emissions from space and related applications. Atmospheric Measurement Techniques, 3(4), 781–811. https://doi.org/10.5194/amt-3-781-2010

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