Controlling the conductivity of amorphous LaAlO3/SrTiO 3 interfaces by in-situ application of an electric field during fabrication

Abstract

Amorphous-LaAlO3/SrTiO3 interfaces present metallic conductivity similar to those found in their all-crystalline counterparts. Here, the conductivity of amorphous-LaAlO3/SrTiO3 interfaces is modified by an external electric field applied in-situ with a biased truncated cone electrode (-10 V ≤ Vbias ≤ 20 V) during film growth. By modulating the charge balance of the arriving plasma species, interfacial conduction of the amorphous-LaAlO3/SrTiO3 heterostructures shifts from metallic to insulating via a semiconducting-like characteristic transport mode. This remarkable behavior is explained by a modification of the Al-ion flux impinging the SrTiO3 surface, which alters the amount of near-interface oxygen vacancies being formed at the SrTiO3 surface. © 2013 AIP Publishing LLC.