We explore the multilevel structure and vibrational couplings of hydrogen bonded O-H stretching transitions in acetic acid dimer using femtosecond 2D-IR photon echo spectroscopy. Anharmonic coupling with low-frequency modes and Fermi resonances with overtone/combination levels dominate the complex ultrafast dynamics.
CITATION STYLE
Huse, N., Bruner, B. D., Cowan, M. L., Dreyer, J., Nibbering, E. T. J., Elsaesser, T., & Miller, R. J. D. (2004). Heterodyne 2D-IR photon echo spectroscopy of multi-level OH stretching coherences in hydrogen bonds. In Springer Series in Chemical Physics (Vol. 79, pp. 407–409). https://doi.org/10.1007/3-540-27213-5_125
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