Bright coherent ultrahigh harmonics in the kev x-ray regime from mid-infrared femtosecond lasers

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Abstract

High-harmonic generation (HHG) traditionally combines ∼100 near-infrared laser photons to generate bright, phase-matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here, we show that by guiding a mid-infrared femtosecond laser in a high-pressure gas, ultrahigh harmonics can be generated, up to orders greater than 5000, that emerge as a bright supercontinuum that spans the entire electromagnetic spectrum from the ultraviolet to more than 1.6 kilo-electron volts, allowing, in principle, the generation of pulses as short as 2.5 attoseconds. The multiatmosphere gas pressures required for bright, phase-matched emission also support laser beam self-confinement, further enhancing the x-ray yield. Finally, the x-ray beam exhibits high spatial coherence, even though at high gas density the recolliding electrons responsible for HHG encounter other atoms during the emission process.

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Popmintchev, T., Chen, M. C., Popmintchev, D., Arpin, P., Brown, S., Ališauskas, S., … Kapteyn, H. C. (2012). Bright coherent ultrahigh harmonics in the kev x-ray regime from mid-infrared femtosecond lasers. Science, 336(6086), 1287–1291. https://doi.org/10.1126/science.1218497

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