Order to disorder in quasiperiodic composites

Abstract

From quasicrystalline alloys to twisted bilayer graphene, the study of material properties arising from quasiperiodic structure has driven advances in theory and applied science. Here we introduce a class of two-phase composites, structured by deterministic Moiré patterns, and we find that these composites display exotic behavior in their bulk electrical, magnetic, diffusive, thermal, and optical properties. With a slight change in the twist angle, the microstructure goes from periodic to quasiperiodic, and the transport properties switch from those of ordered to randomly disordered materials. This transition is apparent when we distill the relationship between classical transport coefficients and microgeometry into the spectral properties of an operator analogous to the Hamiltonian in quantum physics. We observe this order to disorder transition in terms of band gaps, field localization, and mobility edges analogous to Anderson transitions — even though there are no wave scattering or interference effects at play here.