Two-dimensional Raman-echo spectroscopy; femtosecond view of vibrational coherence

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Abstract

Two semiclassical algorithms (high temperature and low temperature, weak nonlinearity) for computing 2D fifth-order Raman spectra are compared. In both cases the response can be described using phase-space wavepackets.

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Piryatinski, A., Chernyak, V., & Mukamel, S. (1998). Two-dimensional Raman-echo spectroscopy; femtosecond view of vibrational coherence. Springer Series in Chemical Physics, 63, 541–543. https://doi.org/10.1007/978-3-642-72289-9_162

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