Abstract
Two-dimensional femtosecond broadband electronic spectroscopy was used to simultaneously probe parallel pathways of energy transfer in the major light harvesting complex of Photosystem II from plants. Sub-100 femtosecond relaxation between delocalized excitonic states on highly coupled clusters of chlorophylls and several hundred femtosecond to picosecond components of relaxation between clusters were observed.
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Schlau-Cohen, G. S., Calhoun, T. R., Engel, G. S., Read, E. L., Ginsberg, N. S., Zigmantas, D., … Fleming, G. R. (2009). Mapping Parallel Pathways of Energy Flow in LHCII with Broadband 2D Electronic Spectroscopy. In Springer Series in Chemical Physics (Vol. 92, pp. 598–600). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_194
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