We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.
CITATION STYLE
Milder, M. T. W., Brüggemann, B., Miller, M., & Herek, J. L. (2009). Coherent Control of the Exciton Dynamics in the FMO Protein. In Springer Series in Chemical Physics (Vol. 92, pp. 448–450). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_145
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