Superconductivity on the border of weak itinerant ferromagnetism in UCoGe

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Abstract

We report the coexistence of ferromagnetic order and superconductivity in UCoGe at ambient pressure. Magnetization measurements show that UCoGe is a weak ferromagnet with a Curie temperature TC=3K and a small ordered moment m0=0.03μB. Superconductivity is observed with a resistive transition temperature Ts=0.8K for the best sample. Thermal-expansion and specific-heat measurements provide solid evidence for bulk magnetism and superconductivity. The proximity to a ferromagnetic instability, the defect sensitivity of Ts, and the absence of Pauli limiting, suggest triplet superconductivity mediated by critical ferromagnetic fluctuations. © 2007 The American Physical Society.

Figures

  • FIG. 1. Magnetic and SC properties of UCoGe sample 2. (a) Magnetization M as a function of T in a field B of 0.01 T. The dashed line extrapolates to m0 0:03 B for T ! 0. The Curie temperature TC 3 K is marked by the dotted vertical line. Left inset: Hysteresis loop M B at T 2 K with coercive field of 0.3 mT. Right inset: Arrott plot of magnetization isotherms at T 2:0, 2.4, 2.8, 3.0, 3.5, and 4.5 K (from top to bottom). (b) ac susceptibility 0ac (left axis) (in B 10 5 T), and resistance R (right axis) as a function of T. The maximum in 0ac and the broad hump in R locate TC. SC for sample 2 is found below 0.61 K in R T and below 0.38 K in 0ac T .
  • FIG. 2. (a) Specific heat divided by temperature c=T versus T in zero magnetic field for sample 2. The idealized transition (dashed line) has a step size c=T 0:014 J=molK2 at TC 3 K. Bulk SC for sample 2 sets in at 0.38 K (measured by 0ac), but the c T data extend down to 0.5 K only. (b) Thermalexpansion coefficient T for sample 3. The large negative contribution below 5 K is due to FM order. The dashed line gives the idealized transition in T with 1:1 10 6 K 1. The total relative length change L=L
  • FIG. 3. Superconducting properties of UCoGe sample 3. (a) ac susceptibility 0ac (left axis) in B 10 5 T and resistance R (right axis). (b) Specific heat divided by temperature c=T as a function of T. Bulk SC occurs below Tonsets 0:66 K (dotted vertical line). Dashed line: Idealized SC transition using an equal entropy construction with a finite value in the SC state of 0:028 J=molK2. (c) Coefficient of linear thermal expansion T . Bulk SC is observed below Tonsets 0:66 K. Dashed line: Idealized sharp transition with Ts 0:45 K. For B 1 T applied along the dilatation direction L=L the SC transition is no longer resolved.
  • FIG. 4. Upper critical field Bc2 determined by the midpoints of the resistive transitions measured in fixed magnetic fields. The solid lines indicate Bc2=dT 7:2 and 5:2 T=K for samples 2 and 3, respectively, and extrapolate to zero field Ts values of 0.30 and 0.60 K.

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CITATION STYLE

APA

Huy, N. T., Gasparini, A., De Nijs, D. E., Huang, Y., Klaasse, J. C. P., Gortenmulder, T., … Löhneysen, H. V. (2007). Superconductivity on the border of weak itinerant ferromagnetism in UCoGe. Physical Review Letters, 99(6). https://doi.org/10.1103/PhysRevLett.99.067006

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