Early Time Vibrationally Hot Ground-State Dynamics in β-Carotene Investigated with Pump-Degenerate Four-Wave Mixing (Pump-DFWM)

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Abstract

Pump-DFWM is used to study the early events in structural and electronicpopulation dynamics of the S2, S1 and hot-S0 states of β-carotene. New evidence to the existence of a long-lived hot-S0 is discussed.

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Buckup, T., Hauer, J., MÖhring, J., & Motzkus, M. (2009). Early Time Vibrationally Hot Ground-State Dynamics in β-Carotene Investigated with Pump-Degenerate Four-Wave Mixing (Pump-DFWM). In Springer Series in Chemical Physics (Vol. 92, pp. 442–444). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_143

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