We probe the dynamics of band gap collapse in the Mott (electronic) insulator ETF2TCNQ and Peierls (structural) insulator K-TCNQ. The collapse of the Mott gap is a purely electronic process occurring within 20 fs. In the Peierls insulator, the gap collapse takes 300 fs, only after a lattice distortion has relaxed.
CITATION STYLE
Wall, S., Brida, D., Ehrke, H. P., Ardavan, A., Bonora, S., Matsusaki, H., … Cavalleri, A. (2009). Clocking the Collapse of a Mott Gap. In Springer Series in Chemical Physics (Vol. 92, pp. 167–169). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-3-540-95946-5_54
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