The simulated characterization and suitability of semiconductor detectors for strontium 90 assay in groundwater

Abstract

This paper examines the potential deployment of a 10 mm × 10 mm × 1 mm cadmium telluride detector for strontium-90 measurement in groundwater boreholes at nuclear decommissioning sites. Geant4 simulation was used to model the deployment of the detector in a borehole monitoring contaminated groundwater. It was found that the detector was sensitive to strontium-90, yttrium-90, caesium-137, and potassium-40 decay, some of the significant beta emitters found at Sellafield. However, the device showed no sensitivity to carbon-14 decay, due to the inability of the weak beta emission to penetrate both the groundwater and the detector shielding. The limit of detection for such a sensor when looking at solely strontium-90 decay was calculated as 323 BqL−1 after a 1-h measurement and 66 BqL−1 after a 24-h measurement. A gallium-arsenide (GaAs) sensor with twice the surface area, but 0.3% of the thickness was modelled for comparison. Using this sensor, sensitivity was increased, such that the limit of detection for strontium-90 was 91 BqL−1 after 1 h and 18 BqL−1 after 24 h. However, this sensor sacrifices the potential to identify the present radionuclides by their end-point energy. Additionally, the feasibility of using flexible detectors based on solar cell designs to maximise the surface area of detectors has been modelled.