Development of nondestructive assay to fuel debris of fukushima daiichi NPP (1): Experimental validation for the application of a self-indication method

Abstract

We have proposed a new concept of the “self-indication method” combined with neutron resonance densitometry (NRD) for nondestructive assaying of the distribution of nuclear materials in the fuel debris of Fukushima Daiichi NPP. To verify the method, we performed experiments using a 46 MeV electron linear accelerator at the Kyoto University Research Reactor Institute. First, we measured the area densities of gold foil 10, 20, 30, 40, and 50 μm thick by area analysis at the 4.9 eV resonance region. It was confirmed that the area densities of the target nuclide can be determined by conventional NRD and the self-indication method within 3 % accuracy, respectively. As the next step, we added a silver foil of 50 μm thickness to a gold foil of 10 μm thickness and measured the area density of the gold foil. It was shown that the contribution from the other nuclide (silver foil) can be remarkably suppressed by applying the self-indication method. Finally, we have demonstrated a nondestructive assay of nuclear material using a mixture composed of a natural uranium foil, sealed minor actinide samples of 237Np and 243Am. The results indicated that the self-indication method is useful for assaying a mixture of materials with high activity such as fuel debris.