A new experimental system for the study of vibrational energy relaxation is presented. Infrared excitation of vibrational modes and probing via anti-Stokes Raman scattering allows the direct observation of vibrational energy transfer between and out of CH-stretching modes with a temporal resolution of approx. 160 fs.
CITATION STYLE
Hartl, I., & Zinth, W. (1998). Ultrafast vibrational energy transfer studied by a novel spectrometer. Springer Series in Chemical Physics, 63, 499–501. https://doi.org/10.1007/978-3-642-72289-9_149
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