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Journal of Materials Chemistry (2010)
- ISSN: 09599428
- ISBN: 0897917782
- DOI: 10.1039/b925751a
- PubMed: 20545327
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Abstract
The resonance Raman spectrum of the simple alkyne bridge in 4,4'-dinitrotolane radical anion shows two distinct bands, providing proof of the solvent-dependent coexistence of charge-localized and -delocalized species. The Raman spectra of normal modes primarily involving the charge-bearing -PhNO(2) units also support the coexistence of two solvent-dependent electronic species. The temperature dependence of the spectra of the bridging unit shows an inverse relationship between the solvent reorganization energy (lambda(s)) and the temperature.
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