Purcell-enhanced dipolar interactions in nanostructures

Abstract

Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level, which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced dipolar interaction of atoms can be enhanced by a dielectric environment. For this Purcell effect, either a cavity or a waveguide can be used. Here, we combine the high densities achievable in thermal atomic vapors with an efficient coupling to a slot waveguide. In contrast to free-space interactions, atoms aligned within the slot exhibit repulsive interactions that are further enhanced by a factor of 8 due to the Purcell effect. The corresponding blueshift of the transition frequency of atoms arranged in the essentially one-dimensional geometry vanishes above the saturation, providing a controllable nonlinearity at the few-photon level. The experimental results are in good agreement with Monte Carlo simulations that include the dielectric environment, dipolar interactions, and motional effects. The results pave the way towards a robust scalable platform for quantum nonlinear optics and all-optical quantum information processing at room temperature.