Personal Exposure and Inhaled Dose Estimation of Air Pollutants during Travel between Albany, NY and Boston, MA

Abstract

Out of eight deaths caused worldwide, one death is caused due to air pollution exposure, making it one of the top global killers. Personal exposure measurement for real-time monitoring has been used for inhaled dose estimation during various modes of workplace commuting. However, dose-exposure studies during long commutes are scarce and more information on inhaled doses is needed. This study focuses on personal exposures to size-fractionated particulate matter (PM1, PM2.5, PM4, PM7, PM10, TSP) and black carbon (BC) inside a bus traveling more than 270 kms on a highway between Albany, NY and Boston, MA. Measurements were also made indoors, outdoors, and while walking in each city. Mean PM (PM1, PM2.5, PM4, PM7, PM10, TSP) and mean BC concentrations were calculated to estimate the inhaled exposure dose. The highest average PM2.5 and PM10 exposures concentrations were 30 ± 12 and 111 ± 193 µg/m3, respectively, during Boston to Albany. Notably, personal exposure to BC on a bus from Albany to Boston (5483 ± 2099 ng/m3 ) was the highest measured during any commute. The average inhaled dose for PM2.5 during commutes ranged from 0.018 µg/km to 0.371 µg/km. Exposure concentrations in indoor settings (average PM2.5 = 37 ± 55 µg/m3, PM10 = 78 ± 82 µg/m3, BC = 5695 ± 1774 ng/m3 ) were higher than those in outdoor environments. Carpeted flooring, cooking, and vacuuming all tended to increase the indoor particulate level. A high BC concentration (1583 ± 1004 ng/m3) was measured during walking. Typical concentration profiles in long-haul journeys are presented.